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The records of the Storrs Agricultural Experiment Station provide information on one of the oldest agricultural experiment and research stations in the United States. The records provide substantial information on the early years of the Experiment Station from 1888 to 1920. The majority of the records consist of correspondence to and from the executive and administrative staff of the station and local farmers and business organizations interested in obtaining information about the station's experiments and research findings.

The collection contains administrative records and historical documents of the Storrs (Connecticut) Congregational Church.

The collection contains the administrative records, correspondence, legal documents, fliers, notes, and publications of the Storrs Draft Information Committee. The records contain information associated with draft counseling, draft resistance, non-violent protest, peace movement groups, and selective service at the University of Connecticut during the Vietnam War.

The Storrs Family Association held its first reunion in 1891 and annually thereafter until at least 1972. This collection consists of Frank H. Storrs genealogical papers and records from the Storrs Family Association.

The collection contains correspondence, reports, membership lists and other pertinent and ephemeral materials concerning the history, organization, and fraternal affiliates of the Storrs School Literary Society (later the College Shakespearean Club).

This collection holds the personal and professional papers of Stuart Saunders Smith including compositions, recordings, correspondence, writings, and photographs.

This collection documents student unrest and activism at the University of Hartford as well as other campuses during the 1960s and 1970s.

The collection contains the original manuscripts of children's author Susan B. Aller as well as her collection of works by J.M. Barrie.