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The papers consist of correspondence, writings, subject files, memorabilia, photographs, financial records, and other papers detailing the professional career and personal life of Anson Phelps Stokes and family members, including Olivia, Caroline and Helen Stokes. Papers relating to Anson Phelps Stokes document his work with prominent educators, reformers, religious leaders, businessmen, and politicians. Stokes's work on behalf of black education, social issues, and the Phelps-Stokes Fund are detailed. His religious activities, Yale University work, and family interests are also represented, as are Stokes's work on behalf of the Portsmouth Treaty of 1905 and the Yale-China Association. Papers relating to Helen Phelps Stokes include material relating to the Socialist Party and the National Civil Liberties Bureau.

The papers consist of correspondence with Edward M. House (1920-1938), personal correspondence, manuscripts and correspondence preparatory to the publication of Seymour's Intimate Papers of Colonel House (1926-1928), newspaper clippings, articles, and memorabilia. Much of the material concerns Seymour's role as delegate to the Paris Peace Conference of 1919.

The papers document three generations of the Woolsey family. The most prominent figures in the collection are William Walton Woolsey (1766-1839), land owner and merchant in New York City; his son, Theodore Dwight Woolsey (1801-1889), Greek scholar, political theorist and president of Yale College; and Theodore Salisbury Woolsey (1852-1929), professor of international law at Yale Law School, son of Theodore Dwight Woolsey. The papers of William Walton Woolsey contain extensive business correspondence, ledgers, legal papers, documents relating to land sales in New York and Ohio, as well as family and personal letters. Since he was engaged in the importation of sugar, cotton and hardware, some of his business correspondence is political with discussions of the Jay Treaty of 1794, the problems of piracy, American neutrality in the 1790s and the general politics of the period. Important correspondents are Chauncey Goodrich, Archibald Gracie, Eli Whitney, Noah Webster, Elihu and Nathaniel Chauncey, Oliver Wolcott, Benjamin Tallmadge, Jedidiah Morse, James Roosevelt, John A. Schuyler, Comfort Sands, John Broome, and Nicholas Bayard. The papers of Theodore Dwight Woolsey contain his writings on Greek language and literature, the Bible, international law and the texts of his sermons.