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The papers consist of correspondence, research files (including notes, transcripts, and photocopies of historical documents), writings, photograph albums, and memorabilia relating to the personal life and professional career of American historian Charles McLean Andrews; his wife, Evangeline Walker Andrews; and other family members. More than half the correspondence is between family members. Charles Andrews's education and early career are detailed in correspondence with his parents, wife, and sisters. Evangeline Andrews's correspondence with her parents; her sister, Ethel Walker Smith; her husband; and her children concerns her Bryn Mawr activities, travels, historical and theatrical interests and writing, and the activities of family members. The correspondence also chronicles the development of the Ethel Walker School. Charles McLean Andrews's professional correspondents include former students, co-authors, fellow historians, librarians, and archivists. The professional correspondence is overwhelmingly incoming and reflects more of the correspondents' careers and activities than those of Andrews. Research and writings files detail Andrews's historical interests.

The papers include correspondence, diaries, scrapbooks, and writings which document Edward G. Bourne's academic career, at Adelbert College and Yale University, historical studies, and professional activities. The papers highlight Bourne's research on Marcus Whitman and his participation on program committees and the Commission on Historical Manuscripts of the American Historical Association.