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The papers consist of correspondence, diaries, writings, research, notes, scrapbooks, and other materials documenting Lounsbury's personal life and professional career as an author and educator of English literature at Yale University. Correspondence with Yale colleagues, students, authors, and officials details his academic and literary interests, and activity in the areas of international language and simplified spelling. Personal materials include letters relating to Lounsbury's Civil War experiences and diaries containing brief entries from 1856-1915.